If the subscription was started through Google Play, it must be cancelled through Google Play, not through LG.
Press the Home button on the LG remote.
Open the LG Content Store.
Select your Profile / Account icon (usually top right).
Go to My Page or Account Management.
Select Purchase History or Subscriptions.
Locate the active subscription.
Select it and choose Cancel.
Go to lg.com.
Sign in to the LG account used on the TV.
Navigate to My Account.
Go to Purchase History or Subscriptions.
Select the subscription and choose Cancel.